By Joshua Jortner, Raphael D. Levine, Stuart Alan Rice

ISBN-10: 047106274X

ISBN-13: 9780471062745

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Extra info for Advances in Chemical Physics (Wiley Series in Probability and Mathematical Statistics)

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Gains, J. K. Kay, and F. M. Page, Trans. , 62,874 (1966). 08. 7 228 ? 23 1752 17 1882 18 Expr. APPLICATION TO NITRIC OXIDE FLUORESCENCE QUENCHING 39 The model also accounts for the trend observed in the CH,Cl,-,(x=O4) series. Introduction of one chlorine atom is expected to lead to a large increase in EA. More chlorine atoms (or deuteration) are expected to have a much smaller effect. Indeed, comparison of CHC1, and CCl, is in line with this contention, as well as the negligible deuteration effect.

60, 1740 (1974). 'A. F. Gains, J. K. Kay, and F. M. Page, Trans. , 62,874 (1966). 08. 7 228 ? 23 1752 17 1882 18 Expr. APPLICATION TO NITRIC OXIDE FLUORESCENCE QUENCHING 39 The model also accounts for the trend observed in the CH,Cl,-,(x=O4) series. Introduction of one chlorine atom is expected to lead to a large increase in EA. More chlorine atoms (or deuteration) are expected to have a much smaller effect. Indeed, comparison of CHC1, and CCl, is in line with this contention, as well as the negligible deuteration effect.

In kinetic studies laser-pumped dye lasers offer both spectral tunability and resolution on the one hand, and good time resolution on the other hand. With typical available dye laser systems (pumped by a nitrogen or a Nd-YAG laser) pulse duration and energy are s and l o p 3J, respectively. Using the data of the above example, about 10" photons are absorbed per laser pulse, creating 5 X lo9 excited molecules. Detection of such small changes in either laser intensity or excited molecule population is a considerable experimental challenge.

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Advances in Chemical Physics (Wiley Series in Probability and Mathematical Statistics) by Joshua Jortner, Raphael D. Levine, Stuart Alan Rice


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